According to Guten Tag! magazine, the couple purchased a luxurious Berlin loft apartment.
A source said: 'Angelina already has homes in the US and an apartment in Paris in France. She and Brad regularly visit Berlin and Angelina is keen that her children should not grow up in Hollywood.' The couple's new apartment is a 6,500 square-foot attic flat near Alexanderplatz square.
Brad already has links with Germany. He is good friends with German architects Lars Krueckeberg, Wolfram Putz and Thomas Willemeit, who designed his Los Angeles house.
He and Angelina recently relocated their family from Hollywood to New Orleans, where they have been looking for good schools for the children.
The couple have two adopted children - Cambodian son Maddox, aged five and two-year-old Ethiopian daughter Zahara.
They also have eight-month-old daughter Shiloh.